Excessive bromine, iodine and dyes can damage soil structure and aquatic ecosystems. Therefore, capturing toxic bromine, iodine and dyes from nuclear fuel waste and organic waste liquid is crucial for protecting the environment and human health. In this study, a tridentate imide acid monomer was synthesized with various functional groups and structures, including carboxyl (-COOH), amide (-CONH), and imide rings, to construct a new type of hyper-crosslinked poly (amide-imide) (PAI1-PAI4). Subsequently, porous carbons (PAI1-900-PAI4900) were prepared, and urea was doped during the secondary carbonization process. The ammonia gas (NH3) and carbon dioxide (CO2) generated from the high-temperature decomposition of urea can be trapped by the porous structure of the carbon-based derivatives, and these gases then react with the carbon in the porous carbon and the N-H/C-H in the amide groups, thus resulting in carbon-based materials (PAI1-U-900-PAI4-U-900) with multiple nitrogen and oxygen Lewis basic sites (C-N/N-O/C--O/-OH) and a moderate porosity. These materials enhanced the interactions between the adsorbent and bromine, iodine, and anionic dyes, and exhibited selective adsorption effects for bromide and Congo red (CR).