We used the GEANT4 toolkit to simulate the altitude and latitude profiles of the production rate of C-14, Be-10 and Cl-36 radionuclides by the galactic cosmic ray (GCR) interactions in the terrestrial atmosphere at a varying geomagnetic field. We found that applying two intranuclear cascade models incorporated in GEANT4 (Binary Intranuclear Cascade, BIC, and Bertini Intranuclear Cascade, BERT) result in significantly different production rate values. We present the conclusions about the certain model relevance to the abundance of these isotopes in the surface fallout, ice-core records and lunar soil depth profile. Comparison of our simulations with the recent publication of Poluianov et al. (2016) shows a good agreement for C-14 (BIC) and Be-10 (BERT) and a definite by the factor 2-3 difference in the Cl-36 (BIC) atmospheric yield functions. Also, the mean level and amplitude of the Be-10 variations in polar ice from central regions of Antarctica and Greenland could be accounted for its tropospheric production by GCRs. The fallout rate of Cl-36 there can be explained assuming its additional input from the stratosphere. Significant additional variations of radionuclide sedimentation rate in polar regions may arise due to tropopause height changes even at a constant atmospheric production rate of the certain isotope.

Stratospheric aerosols cool the Earth by scattering sunlight. Although sulfuric acid dominates the stratospheric aerosol, this study finds that organic material in the lowermost stratosphere contributes 30-40% of the nonvolcanic stratospheric aerosol optical depth (sAOD). Simulations indicate that nonvolcanic sAOD has increased 77% since 1850. Stratospheric aerosol accounts for 21% of the total direct aerosol radiative forcing (which is negative) and 12% of the total aerosol optical depth (AOD) increase from organics and sulfate. There is a larger stratospheric influence on radiative forcing (i.e., 21%) relative to AOD (i.e., 12%) because an increase of tropospheric black carbon warms the planet while stratospheric aerosols (including black carbon) cool the planet. Radiative forcing from nonvolcanic stratospheric aerosol mass of anthropogenic origin, including organics, has not been widely considered as a significant influence on the climate system.