This paper reports the second part of the keynote lecture, whose part I has been already published in this journal, presenting extensive experimental research on the investigation of clay microstructure and its evolution upon loading. Whether the first part focused on the micro to macro behaviour of different reconstituted clays, this part instead concerns the microscale features of the corresponding natural clays, their changes under different loading paths and the ensuing constitutive modelling implications. The experimental investigation is carried out according to the methodology outlined in the part I-paper, hence micro-scale analyses are presented on natural clays subjected to macro-scale mechanical testing, with the purpose to provide experimental evidence of the processes at the micro-scale which underlie the clay response at the macroscale. As for the reconstituted clays in the part I-paper, original results on stiff Pappadai and Lucera clay, this time in their natural state, are compared to literature results on clays of different classes, either soft or stiff. The results presented in this paper, together with those discussed in the part I, allow for a conceptual modelling of the microstructure evolution under compression of natural versus reconstituted multi-mineral clays, providing microstructural insights into the macro-behaviour described by constitutive laws and advising their mathematical formalization in the framework of either continuum mechanics or micro-mechanics.

This keynote lecture discusses the results of a long lasting experimental research, devoted to the investigation of clay microstructure and its evolution upon loading. Micro-scale analyses, involving scanning electron microscopy, image processing, mercury intrusion porosimetry and swelling paths to test the clay bonding, are presented on clays subjected to different loading paths, with the purpose of providing experimental evidence of the processes at the micro-scale which underlie the clay response at the macro-scale. Data from the literature on clays of different classes, either soft or stiff, are compared to original results on two stiff clays, Pappadai and Lucera clay, both in their natural state and after reconstitution in the laboratory. The results presented herein allow building a conceptual model of the evolution of clay microstructure upon different loading paths, providing microstructural insights into the macro-behaviour described by constitutive laws and advising their mathematical formalization in the framework of either continuum mechanics or micro-mechanics. For editorial purposes, the research results are presented in two parts. The first part, presented in this paper, concerns the results for reconstituted clays, whereas a second part, concerning the corresponding natural clays, is discussed in a second companion paper.