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This study investigates aerosol characteristics using ground-based measurements at two distinct regions, MohalKullu (31.9 degrees N, 77.12 degrees E; 1154 m amsl) and Kosi-Katarmal (29.64 degrees N, 79.62 degrees E; 1225 m amsl), from July 2019 to June 2022. The average Black Carbon (BC) concentrations were 1.5 f 1.0 mu g m- 3 at Mohal and 1.1 f 1.4 mu g m-3 at Katarmal. BC showed strong seasonal variability, with maxima during post-monsoon (2.6 f 1.0 mu g m- 3) and pre-monsoon (1.8 f 0.5 mu g m-3) seasons. The diurnal variation displayed distinct morning and evening peaks in all the seasons. High pre-monsoon AOD500 (0.30 f 0.06 to 0.54 f 0.08) and low values of & Aring;ngstrom exponent (0.67 f 0.10 to 0.95 f 0.30) indicated dominance of large particles, whereas lower AOD500 (0.21 f 0.07 to 0.25 f 0.03) in post-monsoon and winter, along with larger & Aring;ngstrom exponent (1.05 f 0.74 to 1.13 f 0.11), indicated smaller particles. Satellite-derived (OMI and MAIAC) AOD500 showed weak to moderate correlation with ground-based measurements at Mohal (R = 0.4639 for MAIAC, R = 0.1402 for OMI) and Katarmal (R = 0.3976 for MAIAC, R = 0.2980 for OMI). Using optical properties of aerosols and clouds (OPAC) and Santa Barbara discrete ordinate radiative transfer (SBDART) models, the short-wave aerosol radiative forcing (SWARF) was found negative at the surface and top of the atmosphere but positive in the atmosphere, suggesting significant surface cooling and atmospheric warming leading to high heating rates, respectively. Annual mean atmospheric radiative forcing was 27.36 f 6.00 Wm- 2 at Mohal and 21.87 f 7.26 Wm- 2 at Katarmal. These findings may have consequences for planning air pollution strategies and understanding the effects of regional climate change.

期刊论文 2025-04-01 DOI: 10.1016/j.jastp.2025.106487 ISSN: 1364-6826

The Black carbon (BC) and Brown carbon (BrC) concentration has been measured over Srinagar (Garhwal) in central Himalayas during October 2020 to September 2021 periods. The average BC mass was 2.59 +/- 1.96 mu g m- 3 and its absorption coefficients were abundant at shorter wavelength. BC seasonal variation exhibited a significant variability, with highest during winter (4.54 +/- 2.64 mu g m- 3) followed by pre-monsoon (2.69 +/- 2.04 mu g m- 3) and post-monsoon (1.93 +/- 0.91 mu g m- 3) while lowest was observed in the monsoon (1.05 +/- 0.54 mu g m- 3). Relatively high contribution of total spectral light absorption coefficient (Abs lambda) was observed (75.94 Mm-1) at 370 nm than longer wavelength (16.86 Mm-1) at 950 nm. The BrC contribution was higher at 370 nm (32.50 Mm-1) to the total babs (lambda), while at higher wavelengths it has extensively decreased (2.54 Mm-1 at 660 nm). Seasonally, the absorption coefficient of BC and BrC was greater in winter (83.99 and 68.37 Mm-1) while lowest in monsoon (19.38 and 9.27 Mm-1), respectively. The babs BrC/babs (t) ratio revealed higher contribution of BrC in winters. The secondary brown carbon (BrCsec) and primary brown carbon (BrCpri) contributed 43.16 % and 56.88 % towards the total BrC Abs (lambda) at 370 nm with higher in winter and lowest in monsoon, respectively. BrCsec and BrCprim has shown higher contribution in evening (18.00-20.00 h) and in morning (09.00-11.00 h) hours. The average radiative forcing (RF) of BC was 36.11 +/- 6.99 Wm-2, 2.19 +/- 1.22 Wm-2 and -33.92 +/- 5.96 Wm-2 at the atmosphere (ATM), Top of the Atmosphere (TOA), and at the Surface (SUR), respectively.

期刊论文 2024-10-01 DOI: 10.1016/j.pce.2024.103670 ISSN: 1474-7065

The NCAR Community Earth System Model is used to study the influences of anthropogenic aerosols on the Indian summer monsoon (ISM). We perform two sets of 30-year simulations subject to the prescribed perpetual SST annual cycle. One is triggered by the year 2000 climatology anthropogenic aerosol emissions data over the Indian Peninsula (referred to as AERO), and the other one is by the year 1850 (referred to as CTL). Only aerosol direct effects are included in the experiments. In our results, the transition of ISM in AERO relative to the CTL exhibits a similar ensemble-mean onset date with a larger spread, and more abrupt onset in late spring, and an earlier but more gradual withdrawal in early fall. The aerosols-induced circulation changes feature an upward motion over the northeastern Indian Peninsula and strengthened anticyclonic circulation over the Arabia Sea in the pre-monsoon season, and a northward shift of monsoon flow in the developed monsoon period along with strengthened local meridional circulation over northern India. The strengthened anticyclonic circulation over Arabia Sea caused a 16% increase in natural dust transport from the Middle East in the pre-monsoon season. The elevated aerosol heating over Tibet causes stronger ascending motion in the pre-monsoon period that leads to earlier and more abrupt ISM onset. The earlier monsoon withdrawal is attributed to the aerosol-induced anticyclonic flow within 10 & DEG;-25 & DEG;N and cyclonic flow within 0 & DEG;-10 & DEG;N over eastern India and Bay of Bengal that resemble the ISM seasonal transition in September.

期刊论文 2023-12-01 DOI: 10.1007/s44195-023-00041-7 ISSN: 1017-0839

In 2015 the beginning of the Indian Smart Cities' mission was one of the significant steps taken by the Indian government to make the urban environment resilient to climate change impact and extreme weather events like drought, floods, heatwaves, etc. This study computes the urban drought risk for Indian smart cities before the beginning of the Indian smart cities mission. This study considers three decadal variability (1982-2013) in meteorological, hydrological, vegetation, and soil moisture parameters for inducing water scarcity and drought conditions in urban regions. Hazards associated with urban drought-inducing parameters variability, vulnerability, and exposure of Indian smart cities were used to compute the Urban drought risk. The research investigations revealed the maximum urban drought risk for Bangalore, Chennai, and Surat cities. Northwest, West Central, and South Peninsular urban regions have higher risk among all the urban regions of India. Indian smart cities mission can be used to make Indian cities resilient to urban drought risk and increase their sustainability. The present research aligned with several national and international agreements by providing an urban drought risk rank for Indian cities, making them less vulnerable to extreme weather events and improving their resilience to climate change.

期刊论文 2023-10-01 DOI: 10.1016/j.jhydrol.2023.130056 ISSN: 0022-1694

This study estimates the radiative forcing by biomass burning and dust aerosols over the Indian subcontinent, with emphasis on the Indo-Gangetic Plains (IGP) during the period from January 2021 to April 2021, based on multiple satellite and reanalysis datasets. In this respect, we used retrievals from the Moderate Resolution Spectroradiometer (MODIS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) system, as well as reanalysis data from the Goddard Earth Observing System, version 5 (GEOS-5), the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2), the Copernicus Atmosphere Monitoring Service (CAMS), and ERA-Interim. According to the MERRA-2 and the CAMS, the highest black carbon (BC) concentrations in January 2021 were 7-8 mu g m(-3), which were significantly lower than measurements performed in main cities along the IGP, such as Patiala, Delhi, and Kanpur. The meteorological data analysis accompanied by the CALIPSO lidar measurements showed that the vertical distribution of total attenuated backscatter (TAB) could reach altitudes of up to similar to 4-5 km and could be transported over the central Himalayan region. The spatial-averaged daily aerosol radiative forcing (ARF) values over the Indian subcontinent from January 2021 to April 2021 were found to range from -51.40 to -6.08 W m(-2) (mean of -22.02 +/- 9.19 W m(-2)), while on a monthly basis, the ARF values varied widely, from -146.24 to -1.63 W m(-2) (mean of -45.56 +/- 22.85 W m(-2)) over different parts of the study region. Furthermore, the spatial-averaged daily BC radiative forcing ranged from -2.23 to -0.35 (-1.01 +/- 0.40 W m(-2)), while it varied from -15.29 to -0.31 W m(-2) (-2.46 +/- 2.32 W m(-2)) over different regions of southern Asia, indicating a rather small contribution to the total aerosol radiative effect and a large presence of highly scattering aerosols. Our findings highlight the importance of growing biomass burning, in light of recent climate change and the rapid decline in air quality over North India and the Indian Ocean.

期刊论文 2023-09-01 DOI: 10.3390/fire6090365 ISSN: 2571-6255

Aerosol-cloud interactions, also known as aerosol indirect effect (AIE), substantially impact rainfall frequency and intensity. Here, we analyze NEX-GDDP, a multimodel ensemble of high-resolution (0.25 degrees) historical simulations and future projections statistically downscaled from 21 CMIP5 models, to quantify the importance of AIE on extreme climate indices, specifically consecutive dry days (CDD), consecutive wet days (CWD), and simple daily intensity index (SDII). The 21 NEX-GDDP CMIP5 models are classified into models with reliable (REM) and unreliable (UREM) monsoon climate simulated over India based on their simulations of the climate indices. The REM group is further decomposed based on whether the models represent only the direct (REMADE) or the direct and indirect (REMALL) aerosol effects. Compared to REMADE, including all aerosol effects significantly improves the model skills in simulating the observed historical trends of all three climate indices over India. Specifically, AIE enhances dry days and reduces wet days in India in the historical period, consistent with the observed changes. However, by the middle and end of the 21st century, there is a relative decrease in dry days and an increase in wet days and precipitation intensity. Moreover, the REMALL simulated future CWD and CDD changes are mostly opposite to those in REMADE, indicating the substantial role of AIE in the future projection of dry and wet climates. These findings underscore the crucial role of AIE in future projections of the Indian hydroclimate and motivate efforts to accurately represent AIE in climate models. We investigate the impacts of aerosol on India's wet and dry climate. High-resolution downscaled CMIP5 models were used to calculate extreme indices like CDD (consecutive dry days), CWD (consecutive wet days), SDII (precipitation intensity). From the group of 22 models, 12 reliable models were chosen based on their fidelity to the observations. Amongst the reliable models, certain models incorporate only aerosol-radiation interaction (REMADE), while others have both aerosol-radiation and aerosol-cloud interaction (REMALL). We found that the simulated trends in the REMAll were similar to the observed trends. In the current period (1975-2005), the aerosol-cloud interactions led to the reduction in rainfall (both frequency and intensity wise) and enhanced the dry days, however in the future projections, the reduction in aerosol emissions leads to a wetter climate (increase in wet days and rainfall intensity) over India.

期刊论文 2023-08-01 DOI: 10.1029/2022EF003266

For the period 2001-2020, the interannual variability of the normalized difference vegetation index (NDVI) is investigated in connection to Indian summer monsoon rainfall (ISMR). According to Moderate Resolution Imaging Spectroradiometer (MODIS) NDVI data, the ISMR and the vegetative activity of the Indo-Gangetic plain (IGP) in the month of January show a significant negative association. We hypothesized that the January vegetation state affects the ISMR via a delayed hydrological response, in which the wet soil moisture anomaly formed throughout the winter to accommodate the water needs of intensive farming influences the ISMR. The soil moisture anomalies developed in the winter, particularly in the root zone, persisted throughout the summer. Evaporative cooling triggered by increasing soil moisture lowers the summer surface temperature across the IGP. The weakening of monsoon circulation as a result of the reduced intensity of land-sea temperature contrast led in rainfall suppression. Further investigation shows that moisture transport has increased significantly over the past two decades as a result of increasing westerly over the Arabian Sea, promoting rainfall over India. Agriculture activities, on the other hand, have resulted in greater vegetation in India's northwest and IGP during the last two decades, which has a detrimental impact on rainfall processes. Rainfall appears to have been trendless during the last two decades as a result of these competing influences. With a lead time of 5 months, this association between January's vegetation and ISMR could be one of the potential predictors of seasonal rainfall variability.

期刊论文 2023-04-01 DOI: 10.1007/s00382-022-06426-7 ISSN: 0930-7575

Variations in annual accumulated snowfall over the Antarctic ice sheet have a significant and direct impact on mean sea-level change. The interannual variability of the precipitation over coastal Antarctica adjacent to the southern Indian Ocean (SIO) cannot be totally explained by the dominant mode of atmospheric variability in the Southern Hemisphere. This study explores the possible contributions from sea surface temperature (SST) anomalies in SIO on the precipitation over East Antarctica. The results suggest that the winter precipitation in the Lambert Glacier basin (LGB) is closely related to the autumn SST variability in SIO without the influence of El Nino-Southern Oscillation. It is shown that the positive autumn SIO dipole (SIOD) of SST anomalies is usually followed by reduced precipitation in the following winter over the LGB region and vice versa. The positive (negative) autumn SIOD can persist into the winter and excite cyclonic (anticyclonic) circulation and deepen (weaken) SIO low in high latitude, corresponding to an enhanced northward (southward) wind anomaly in LGB and central SIO. This mechanism prevents (promotes) the transportation of warm and moist marine air to the LGB region and hence decreases (increases) the precipitation during the following winter.

期刊论文 2022-12-01 DOI: http://dx.doi.org/10.3389/feart.2022.920245

Atmospheric aerosols are very crucial from air pollution and health perspective as well as for regional and global climate. This paper attempts to summarize the aerosol loading and their properties such as Aerosol Optical Depth (AOD), Single Scattering Albedo (SSA), Angstrom exponent, and Radiative forcing, over India. All the above mentioned parameters have shown significant variability with change in the site and season. From various studies it was observed that AOD is relatively higher over Northern part of India as compared to Southern and Eastern part. Generally, lower values of SSA were observed over all sites during winter and post-monsoon seasons which indicates the dominance of absorbing type aerosol during these seasons. Also the ARF within atmosphere showed comparatively higher values during November-December and lower value during August and September all over the India. The current state of knowledge about aerosol sources, interactions and their effects on environment is limited because of its complexity. Therefore, more focused research in needed to understand the aerosol's role in climatic phenomenon.

期刊论文 2022-01-01 DOI: 10.22059/POLL.2021.327809.1146 ISSN: 2383-451X

The COVID-19 lockdown restrictions influenced global atmospheric aerosols. We report aerosol variations over India using multiple remote sensing datasets [Moderate Resolution Imaging Spectroradiometer (MODIS), Ozone Monitoring Instrument (OMI), Cloud-Aerosol Lidar, and Infrared Pathfinder (CALIPSO)], and model reanalysis [Copernicus Atmosphere Monitoring Service (CAMS)] during the lockdown implemented during the COVID-19 pandemic outbreak period from March 25 to April 14, 2020. Our analysis shows that, during this period, MODIS and CALIPSO showed a 30-40% reduction in aerosol optical depth (AOD) over the Indo-Gangetic Plain (IGP) with respect to decadal climatology (2010-2019). The absorbing aerosol index and dust optical depth measurements also showed a notable reduction over the Indian region, highlighting less emission of anthropogenic dust and also a reduced dust transport from West Asia during the lockdown period. On the contrary, central India showed an similar to 12% AOD enhancement. CALIPSO measurements revealed that this increase was due to transported biomass burning aerosols. Analysis of MODIS fire data product and CAMS fire fluxes (black carbon, SO2, organic carbon, and nitrates) showed intense fire activity all over India but densely clustered over central India. Thus, we show that the lockdown restrictions implemented at the government level have significantly improved the air quality over northern India but fires offset its effects over central India. The biomass-burning aerosols formed a layer near 2-4 km (AOD 0.08-0.1) that produced heating at 3-4 K/day and a consequent negative radiative forcing at the surface of similar to-65 W/m(2) (+/- 40 W/m(2)) over the central Indian region.

期刊论文 2021-09-20 DOI: 10.3389/fenvs.2021.746090
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