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This study shows the impact of black carbon (BC) aerosol atmospheric rivers (AAR) on the Antarctic Sea ice retreat. We detect that a higher number of BC AARs arrived in the Antarctic region due to increased anthropogenic wildfire activities in 2019 in the Amazon compared to 2018. Our analyses suggest that the BC AARs led to a reduction in the sea ice albedo, increased the amount of sunlight absorbed at the surface, and a significant reduction of sea ice over the Weddell, Ross Sea (Ross), and Indian Ocean (IO) regions in 2019. The Weddell region experienced the largest amount of sea ice retreat (similar to 33,000 km(2)) during the presence of BC AARs as compared to similar to 13,000 km(2) during non-BC days. We used a suite of data science techniques, including random forest, elastic net regression, matrix profile, canonical correlations, and causal discovery analyses, to discover the effects and validate them. Random forest, elastic net regression, and causal discovery analyses show that the shortwave upward radiative flux or the reflected sunlight, temperature, and longwave upward energy from the earth are the most important features that affect sea ice extent. Canonical correlation analysis confirms that aerosol optical depth is negatively correlated with albedo, positively correlated with shortwave energy absorbed at the surface, and negatively correlated with Sea Ice Extent. The relationship is stronger in 2019 than in 2018. This study also employs the matrix profile and convolution operation of the Convolution Neural Network (CNN) to detect anomalous events in sea ice loss. These methods show that a higher amount of anomalous melting events were detected over the Weddell and Ross regions. Impact Statement Sea ice protects ice sheets, which are melting at a very high rate to raise the sea level. In addition to global warming, this study is indicative that black carbon aerosols transported from anthropogenic wildfire events, such as from the Amazon, darken the snow, reduce their reflectance, increase the absorption of solar energy incident on the surface, and exacerbate the sea ice retreat. Thus, this study points out that anthropogenic wildfire impacts far away from a region can have a severe impact on sea ice and ice sheets over the Antarctic which has a sea level rise potential of 60 m. Our study shows that only over the Weddell region, sea ice retreat was 20,000 km(2) higher during the presence of BC transport events than other days in 2019.

期刊论文 2025-01-01 DOI: 10.1017/eds.2025.1

An extreme biomass burning event occurred in the Amazonian rainforest from July through September 2019 due to the extensive wildfires used to clear the land, which allowed for more significant forest burning than previously occurred. In this study, we reclustered the clear-sky ambient aerosols to adapt the black carbon (BC) aerosol retrieval algorithm to Amazonia. This not only isolated the volumetric fraction of BC (f(bc)) from moderate-resolution imaging spectroradiometer (MODIS) aerosol data, but also facilitated the use of aerosol mixing and scattering models to estimate the absorption properties of smoke plumes. The retrieved MODIS aerosol dataset provided a space perspective on characterizing the aerosol changes and trends of the 2019 pollution event. A very high aerosol optical depth (AOD) was found to affect the source areas continuously, with higher and thus stronger aerosol absorption. These pollutants also affected the atmosphere downwind due to the transport of air masses. In addition, properties of aerosols emitted from the 2019 Amazonian wildfire events visualized a significant year-to-year enhancement, with the averaged AOD at 550 nm increased by 150%. A 200% increase in the aerosol-absorption optical depth (AAOD) at 550 nm was recognized due to the low single-scattering albedo (SSA) caused by the explosive BC emissions during the pollution peak. Further simulations of aerosol radiative forcing (ARF) showed that the biomass-burning aerosols emitted during the extreme Amazonian wildfires event in 2019 forced a significant change in the radiative balance, which not only produced greater heating of the atmospheric column through strong absorption of BC, but also reduced the radiation reaching the top-of-atmosphere (TOA) and surface level. The negative radiative forcing at the TOA and surface level, as well as the positive radiative forcing in the atmosphere, were elevated by similar to 30% across the whole of South America compared to 2018. These radiative effects of the absorbing aerosol could have the ability to accelerate the deterioration cycle of drought and fire over the Amazonian rainforest.

期刊论文 2022-05-01 DOI: 10.3390/rs14092080
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