["Patel, Piyushkumar N","Dumka, U. C","Babu, K. N","Mathur, A. K"]2017-12-01期刊论文
Long-term measurements of spectral aerosol optical depth (AOD) using sun/sky radiometer for a period of five years (2009-2014) from the remote island location at Kavaratti (KVT; 10.56 degrees N, 72.64 degrees E) in the southern Arabian sea have been analysed. Climatologically, AODs decrease from October to reach maximum of similar to 0.6 (at 500nm) in March, followed by a sudden fall towards May. Significant modulations of intra-seasonal timescales over this general pattern are noticed due to the changes in the relative strength of distinctively different sources. The corresponding changes in aerosol inversion parameters reveal the presence of coarse-mode aerosols during spring and fine-mode absorbing aerosols in autumn and winter months. An overall dominance of a mixed type of aerosols (similar to 41%) with maximum in winter (similar to 53%) was found via the AOD(500) vs. Angstrom exponent (alpha(440-870)) relationship, while biomass-burning aerosols or thick urban/industrial plumes contribute to similar to 19%. Spectral dependence of Angstrom exponent and aerosol absorbing properties were used to identify the aerosol types and its modification processes. Based on air mass back trajectory analysis, we revealed that the advection of aerosols from Indian subcontinent and western regions plays a major role in modifying the optical properties of aerosols over the observational site. The shortwave aerosol direct radiative forcing estimated via SBDART model ranges from -11.00 W m(-2) to -7.38 W m(-2), -21.51 W m(-2) to -14.33 W m(-2) and 3.17 W m(-2) and 10.0 W m(-2) at top of atmosphere, surface and within the atmosphere, respectively. This atmospheric forcing translates into heating rate of 0.62-1.04 K day(-1). Furthermore, the vertical profiles of aerosols and heating rate exhibit significant increase in lower (during winter and autumn) and mid troposphere (during spring). This may cause serious climate implications over Kavaratti with further consequences on cloud microphysics and monsoon rainfall. (C) 2017 Elsevier B.V. All rights reserved.
